Conclusions We simulated the photoluminescence spectra of vertically grown pairs of quantum dots and observed that their size is a crucial factor to achieve coupling via magnetic field. Two sets of dots were examined: the first one does not couple because its dimensions selleck screening library strengthen Coulomb interaction and disfavors diamagnetic shift. In contrast, the second one with larger dimensions exhibits a very different behavior as the magnetic field increases, showing the characteristic anticrossings of molecular coupling. The
presence of coupling is highly affected by the Coulomb interaction, regardless of the fact that its value is around 2 orders of magnitude smaller than the exciton energy. Moderate-low temperature (below the nitrogen boiling point) was found enough
to optically observe excited states, which is directly related to the small gap between hybridized states in the resonance region. From these results, we conclude that magnetically tuned tunneling coupling eases optical observation of excited states as compared to single-dot states. Furthermore, effective control on the energy, polarization, and intensity of emitted light, through externally applied magnetic field, has been shown which suggests that this type of on-demand coupled nanostructures BKM120 solubility dmso is a relevant candidate for the implementation of quantum optoelectronic devices. Endnotes a For the electron (hole) g factor, we used −0.745 (−1.4). b The following parameters were used in the calculations: InAs (GaAs) eletron mass 0.023 m e (0.067 m e ), InAs (GaAs) hole mass 0.34 m e (0.34 m e ), and InAs (GaAs) confinement potential V 0=474 meV (258 meV). c Although the
top dot is larger than the bottom one, because of its heaviness, the hole has similar eigenenergies in each of them, and vertical strain effects (as reported in [14]) are likely to be more relevant than those of size. Thus, we assume the ground hole state to remain in the bottom Montelukast Sodium dot. d An interband gap of 800 meV was used in our calculations. Authors’ information NRF is a MSc degree selleck chemicals holder and is a lecturer in the Physics Department of UAN. ASC is a Ph.D. degree holder and is a Senior Researcher and Professor in Universidad de Los Andes. HYR is a Ph.D. degree holder and is an Assistant Professor in the School of Physics of UPTC. Acknowledgements This work was financially supported by the Department of Physics of Universidad de Los Andes and the Research Division of UPTC. References 1. Doty MF, Scheibner M, Bracker AS, Gammon D: Optical spectroscopy of spins in coupled quantum dots . In Nanoscience and Technology. Volume 1. Edited by: Michler P. Berlin: Springer; 2009:330–366. 2. Krenner HJ, Sabathil M, Clark EC, Kress A, Bichler M, Abstreiter G, Finley JJ: Direct observation of controlled coupling in an individual quantum dot molecule . Phys Rev Lett 2005, 94:057402. 15783693CrossRef 3. Voskoboynikov O: Theory of diamagnetism in asymmetrical vertical quantum dot molecule .